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| 標題: | Fixed-bed adsorption of copper from aqueous media using chitosan-coated bentonite, chitosan-coated sand, and chitosan-coated kaolinite |
| 作者: | Futalan, Cybelle M.
Yang, Jung-Hung
Phatai, Piaw
Chen, I-Pin
Wan, Meng-Wei |
| 貢獻者: | Dong A Univ, Natl Res Ctr Disaster Free & Safe Ocean City
Chia Nan Univ Pharm & Sci, Dept Environm Engn & Sci
Udon Thani Rajabhat Univ, Dept Chem, Fac Sci
Chia Nan Univ Pharm & Sci, Dept Environm Resources Management |
| 關鍵字: | Breakthrough curve
Chitosan
Clay
Fixed-bed
Mass transfer zone
Sand
Thomas model |
| 日期: | 2020 |
| 上傳時間: | 2022-11-18 11:26:16 (UTC+8) |
| 出版者: | Springer Heidelberg |
| 摘要: | Fixed-bed studies were performed to evaluate the removal efficiency of copper (Cu(II)) from aqueous solution using chitosan-coated bentonite (CCB), chitosan-coated sand (CCS), and chitosan-coated kaolinite (CCK). The thermal and morphological properties of CCB, CCK, and CCS were characterized using thermogravimetric analysis, Fourier transform infrared spectroscopy, and the Brunauer-Emmett-Teller method. Dynamic experiments were carried out to investigate the effect of solution pH (3.0 to 5.0) and initial Cu(II) concentration (200 to 1000 mg/L) on the time to reach breakthrough (t(b)), total volume of treated effluent (V-eff), and adsorption capacity at breakthrough (q(b)). Results show that increasing the initial Cu(II) concentration inhibits the column performance where lowerV(eff),t(b), andq(b)were obtained. Decreasing the pH from 5.0 to 3.0 led to improved removal efficiency with higher values ofV(eff),t(b), andq(b). Under pH 3.0 and 200 mg/L, the maximum removal efficiency of 68.60%, 56.10%, and 58.90% for Cu(II) was attained using CCB, CCS, and CCK, respectively. The Thomas model was determined to adequately predict the breakthrough curves based on high values of coefficient of determination (R-2 >= 0.8503). Regeneration studies were carried out using 0.1 M HCl and 0.1 M NaOH solution in the saturated column of CCB, CCK, and CCS. |
| 關聯: | Environmental Science and Pollution Research, v.27, n.20, pp.12 |
| 顯示於類別: | [環境工程與科學系(所)] 期刊論文
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