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    题名: Removal of copper, nickel, lead, and zinc using chitosan-coated montmorillonite beads in single- and multi-metal system
    作者: Tsai, Wan-Chi
    Ibarra-Buscano, Sonia
    Kan, Chi-Chuan
    Futalan, Cybelle Morales
    Dalida, Maria Lourdes P.
    Wan, Meng-Wei
    贡献者: Kaohsiung Med Univ, Dept Med Lab Sci & Biotechnol
    Univ Philippines Diliman, Dept Chem Engn
    Chia Nan Univ Pharm & Sci, Inst Hot Spring Ind
    Frontier Oil Corp, Operat Dept
    Chia Nan Univ Pharm & Sci, Dept Environm Engn & Sci
    关键词: Ionic strength
    Multi-metal system
    Chitosan
    Groundwater
    Hydrated ionic radius
    water
    日期: 2016-05
    上传时间: 2018-01-18 11:39:59 (UTC+8)
    出版者: Taylor & Francis Inc
    摘要: In this study, the removal of Cu(II), Ni(II), Pb(II), and Zn(II) from aqueous solution in single and multi-metal system using chitosan-coated montmorillonite (ChiMC) beads was investigated. The non-crosslinked and crosslinked ChiMC beads were characterized using SEM-EDX, Fourier transform infrared, and Brunauer, Emmett, and Teller analysis. The effect of ionic strength and pH on the adsorption capacity and percent (%) removal of ChiMC was examined. Kinetic studies revealed that adsorption using ChiMC follows the pseudo-second-order equation with high correlation coefficient values (R-2>0.95). The equilibrium data were correlated with Langmuir and Freundlich isotherm models, where crosslinked ChiMC provided higher maximum adsorption capacity over ChiMC. The calculated Langmuir adsorption capacities for Cu(II), Ni(II), Pb(II), and Zn(II) using ChiMC in single-metal system are 13.04, 12.18, 29.85, and 13.50mg/g, respectively. An increase in the calculated adsorption capacities derived from Langmuir isotherm was observed in multi-metal system, indicating a synergistic effect. The adsorption capacity in single- and multi-metal system followed the order: Pb(II)>Cu(II)>Zn(II)>Ni(II). The kinetic rate and adsorption capacity of the four metals were observed to increase in multi-metal systems. The removal of Cu(II), Ni(II), Pb(II), and Zn(II) from groundwater by adsorption onto ChiMC was also investigated.
    關聯: Desalination and Water Treatment, v.57 n.21, pp.9799-9812
    显示于类别:[Dept. of Environmental Engineering and Science (including master's program)] Periodical Articles
    [Dept. of Tourism Management] Periodical Articles

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